Anchoring Ag3PO4 nanoparticles on MIL-101(Fe)@nanocellulose composite for tetracycline degradation

Nguyen Thi Hoa; Le Thi Nguyen; Vu Van Tai; Pham Xuan Nui

doi:10.51316/jca.2021.079

Authors

Nguyen Thi Hoa Deparment of Chemical Engineering, Hanoi University of Mining and Geology Author
Le Thi Nguyen Deparment of Chemical Engineering, Hanoi University of Mining and Geology Author
Vu Van Tai Department of Chemical Engineering, Hanoi University of Mining and Geology Author
Pham Xuan Nui Department of Chemical Engineering, Hanoi University of Mining and Geology Author

DOI:

https://doi.org/10.51316/jca.2021.079

Keywords:

Photocatalyst, Nanocellulose (NC), Ag3PO4@MIL-101(Fe)@NC, Tetracycline (TC)

Abstract

In this research, the combination of the photocatalytic activity of the semiconductor Ag₃PO₄ and the as-synthesized MIL-101(Fe)@nanocellulose (NC) from agricultural and bottle waste sources exhibited great photocatalytic efficiency. The Ag₃PO₄@MIL-101(Fe)@nanocelllulose (NC) composite has overcome the disadvantages of pure Ag₃PO₄ and significantly improved the photocatalytic activity. Structural characteristics, morphology of the materials were analyzed by X-ray diffraction (XRD), scanning electron microscopy (SEM), energy dispersive X-ray spectroscope (EDX), and UV–vis diffuse reflectance spectroscopy (UV-vis DRS) methods. From the obtained results, composite has a narrow bandgap energy (2.45 eV) and excellent catalytic performance in the photodegradation of Tetracycline pollutants (99.7 % after 120 min). It demonstrates the development of new catalysts made from agricultural waste sources that show high stability, ease of fabrication and can operate in natural light for environmental remediation.

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