Surface characterization and oxygen electroreduction of self-assembled porphyrin monolayer electrodeposited on copper single crystal electrode
Abstract
A novel approach supported for the enhancement of the oxygen electroreduction activity via self-assembled monolayer of porphyrin (TAP) electrodeposited on Cu (100) electrode surface is demonstrated. While the electrochemical response and surface structure at the molecular level of the TAP monolayer are characterized upon employing combined cyclic voltammetry (CV) and in-situ electrochemical scanning tunneling microscopy (EC-STM) its electrocatalytic activity is revealed by using linear sweep voltammetry (LSV). The LSV results show that this self-assembled monolayer enables significant enhancement the oxygen electroreduction. This finding opens a new approach to improve the efficiency of the oxygen electroreduction using organic molecular self-assemblies.
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